Stratified sampling procedure was employed to collect a total of 40 samples; 2 from each stratum, measuring an approximate dimension of 3.25 km(2) of the actual sample site. Appropriate volumes were then evaporated and transferred into clean stainless steel planchets (ISO 9696 and ISO 9697). An eight channel gas-flow proportional counting system connected to a microprocessor loaded with a spreadsheet programme (Quarttro-Pro) and graphic programme (Multiplan) initially calibrated for efficiency was employed to count the background and the prepared samples. A mean efficiency of 33.44 and 41.24 % for the respective alpha and beta sources was obtained. A low background activity was also observed with a mean of 0.165 Bq for alpha and 1.119 Bq for beta. The gross alpha and beta activity concentrations in the water were found to range from 80 +/- 0.05 to 2300 +/- 0.41 Bq m(-3) and 120 +/- 0.08 to 4970 +/- 0.78 Bq m(-3), respectively. This clearly indicate areas of elevated alpha and beta activity concentrations of 37.5 and 47.5 %, respectively when compared with the International Commission for Radiological Protection (1991) maximum acceptable values of 500 Bq m(-3) for alpha and 1000 Bq m(-3) for beta.
Measurements of (222)Rn activity concentration were carried out in 39 samples collected from the domestic and drinking water sources used in the island and mainland of Penang, northern peninsular, Malaysia. The measured activity concentrations ranged from 7.49 to 26.25 Bq l(-1), 0.49 to 9.72 Bq l(-1) and 0.58 to 2.54 Bq l(-1) in the raw, treated and bottled water samples collected, respectively. This indicated relatively high radon concentrations compared with that from other parts of the world, which still falls below the WHO recommended treatment level of 100 Bq l(-1). From this data, the age-dependent associated committed effective doses due to the ingestion of (222)Rn as a consequence of direct consumption of drinking water were calculated. The committed effective doses from (222)Rn resulting from 1 y's consumption of these water were estimated to range from 0.003 to 0.048, 0.001 to 0.018 and 0.002 to 0.023 mSv y(-1), for age groups 0-1, 2-16 and >16 y, respectively.