Roasted flaxseed is a viable food for augmenting ω-3 fatty acid intake; however, their sticky mouthfeel limits broader acceptance. The relationship between flaxseed components and sensory properties remains underexplored. This study compares sensory attributes of several flaxseed cultivars and investigates the correlation between changes in composition and sensory characteristics. Flaxseed mucilage was reduced through extraction, and the effects of different roasting conditions on physical (moisture, hardness, crispness) and chemical properties (cyclolinopeptides, flax lignans, oxidative indices) were examined. Optimal roasting conditions were identified as 160 °C for 20 min, as identified through principal component analysis. Results indicated that the mucilage layer negatively affected mouthfeel, while cyclolinopeptide E and lignans impacted flavor and aroma. Degumming improved mouthfeel but reduced oxidative stability, suggesting partial degumming for optimized sensory quality and shelf life. This study provides insights into enhancing the sensory experience of roasted flaxseeds without compromising nutritional benefits and oxidative stability.