Affiliations 

  • 1 School of Materials and Mineral Resources Engineering, Universiti Sains Malaysia, Nibong Tebal Penang, 14300, Malaysia; MIND-IN2UB, Department of Electronics and Biomedical Engineering, University of Barcelona, Spain; Institute of Electronics and Photonics, Slovak University of Technology, Ilkovicova 3, Bratislava, 81219, Slovakia
  • 2 Institute of Electronics and Photonics, Slovak University of Technology, Ilkovicova 3, Bratislava, 81219, Slovakia
  • 3 Smart, Advanced Memory Devices and Applications (SAMA) Laboratory, Electrical and Computer Engineering Program, Computer Electrical Mathematical Science and Engineering Division, King Abdullah University of Science and Technology (KAUST), Thuwal, 23955, Kingdom of Saudi Arabia
  • 4 School of Materials and Mineral Resources Engineering, Universiti Sains Malaysia, Nibong Tebal Penang, 14300, Malaysia. Electronic address: mariatti@usm.my
Chemosphere, 2024 Nov;367:143618.
PMID: 39490758 DOI: 10.1016/j.chemosphere.2024.143618

Abstract

Nitrogen dioxide (NO2) is a major cause of respiratory disorders in outdoor and indoor environments. Real-time NO2 monitoring using nonintrusive wearable devices can save lives and provide valuable health data. This study reports a room-temperature, wearable, and flexible smart NO2 gas sensor fabricated via cost-effective printing technology on a polyimide substrate. The sensor uses alkali lignin with edge-oxidised graphene oxide (EGO-AL) ink, demonstrating a sensitivity of 1.70% ppm⁻1 and a detection limit of 12.70 ppb, with excellent selectivity towards NO2. The high sensing properties are attributed to labile oxygen functional groups from GO and alkali lignin, offering abundant interacting sites for NO2 adsorption and electron transfer. The sensor fully recovers to the baseline after heat treatment at 150 °C, indicating its reusability. Integration into lab coats showcased its wearable application, utilising a flexible printed circuit board to wirelessly alert the wearer via cell phone to harmful NO2 levels (>3 ppm) in the environment. This smart sensing application underscores the potential for practical, real-time air quality monitoring, personal safety enhancement, and health management.

* Title and MeSH Headings from MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine.