Affiliations 

  • 1 Department of Chemistry, Faculty of Science, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia. Electronic address: zettyazalea@yahoo.com
  • 2 Department of Chemistry, Faculty of Science, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia
  • 3 Department of Chemistry, Faculty of Science, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia; Centre for Sustainable Nanomaterials, Ibnu Sina Institute for Scientific and Industrial Research, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia. Electronic address: marsin@kimia.fs.utm.my
  • 4 Department of Chemistry, Faculty of Science, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia; Centre for Sustainable Nanomaterials, Ibnu Sina Institute for Scientific and Industrial Research, Universiti Teknologi Malaysia, 81310 UTM Johor Bahru, Johor, Malaysia
Int J Biol Macromol, 2020 Jun 15;153:513-522.
PMID: 32142849 DOI: 10.1016/j.ijbiomac.2020.03.015

Abstract

A new crosslinked chitosan grafted with methyl methacrylate (M-CTS) adsorbent was synthesized via free radical polymerization for effective removal of Cu(II) ions from aqueous solution. Crosslinked chitosan (1 g) was grafted with 29.96 × 10-1 M methyl methacrylate in the presence of 2.63 × 10-1 M ammonium persulfate as initiator at 60 °C for 2 h to give grafting and yield percentages of 201% and 67%, respectively. Batch adsorption experiment was performed as a function of solution pH, initial metal ion concentration and contact time. The isotherm data were adequately described by Langmuir model, while kinetic study revealed that the pseudo-second order rate model best fitted for the experimental data. The maximum adsorption capacity for M-CTS at pH 4 was 192.31 mg g-1. Furthermore, the reusability of over six adsorption-desorption cycles suggested that M-CTS is a durable adsorbent and good candidate for metal ions treatment.

* Title and MeSH Headings from MEDLINE®/PubMed®, a database of the U.S. National Library of Medicine.