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  1. Review on applications of artificial intelligence methods for dam and reservoir-hydro-environment models
    Allawi MF, Jaafar O, Mohamad Hamzah F, Abdullah SMS, El-Shafie A
    Environ Sci Pollut Res Int, 2018 May;25(14):13446-13469.
    PMID: 29616480 DOI: 10.1007/s11356-018-1867-8
    Efficacious operation for dam and reservoir system could guarantee not only a defenselessness policy against natural hazard but also identify rule to meet the water demand. Successful operation of dam and reservoir systems to ensure optimal use of water resources could be unattainable without accurate and reliable simulation models. According to the highly stochastic nature of hydrologic parameters, developing accurate predictive model that efficiently mimic such a complex pattern is an increasing domain of research. During the last two decades, artificial intelligence (AI) techniques have been significantly utilized for attaining a robust modeling to handle different stochastic hydrological parameters. AI techniques have also shown considerable progress in finding optimal rules for reservoir operation. This review research explores the history of developing AI in reservoir inflow forecasting and prediction of evaporation from a reservoir as the major components of the reservoir simulation. In addition, critical assessment of the advantages and disadvantages of integrated AI simulation methods with optimization methods has been reported. Future research on the potential of utilizing new innovative methods based AI techniques for reservoir simulation and optimization models have also been discussed. Finally, proposal for the new mathematical procedure to accomplish the realistic evaluation of the whole optimization model performance (reliability, resilience, and vulnerability indices) has been recommended.
    Matched MeSH terms: Water; Water Resources/supply & distribution*
  2. Technical feasibility study of a low-cost hybrid PAC-UF system for wastewater reclamation and reuse: a focus on feedwater production for low-pressure boilers
    Amosa MK, Jami MS, Alkhatib MF, Majozi T
    Environ Sci Pollut Res Int, 2016 Nov;23(22):22554-22567.
    PMID: 27557958
    This study has applied the concept of the hybrid PAC-UF process in the treatment of the final effluent of the palm oil industry for reuse as feedwater for low-pressure boilers. In a bench-scale set-up, a low-cost empty fruit bunch-based powdered activated carbon (PAC) was employed for upstream adsorption of biotreated palm oil mill effluent (BPOME) with the process conditions: 60 g/L dose of PAC, 68 min of mixing time and 200 rpm of mixing speed, to reduce the feedwater strength, alleviate probable fouling of the membranes and thus improve the process flux (productivity). Three polyethersulfone ultrafiltration membranes of molecular weight cut-off (MWCO) of 1, 5 and 10 kDa were investigated in a cross-flow filtration mode, and under constant transmembrane pressures of 40, 80, and 120 kPa. The permeate qualities of the hybrid processes were evaluated, and it was found that the integrated process with the 1 kDa MWCO UF membrane yielded the best water quality that falls within the US EPA reuse standard for boiler-feed and cooling water. It was also observed that the permeate quality is fit for extended reuse as process water in the cement, petroleum and coal industries. In addition, the hybrid system's operation consumed 37.13 Wh m(-3) of energy at the highest applied pressure of 120 kPa, which is far lesser than the typical energy requirement range (0.8-1.0 kWh m(-3)) for such wastewater reclamation.
    Matched MeSH terms: Water Quality; Waste Water*
  3. Microplastic emissions from household washing machines: preliminary findings from Greater Kuala Lumpur (Malaysia)
    Praveena SM, Syahira Asmawi M, Chyi JLY
    Environ Sci Pollut Res Int, 2021 Apr;28(15):18518-18522.
    PMID: 32935209 DOI: 10.1007/s11356-020-10795-z
    Microplastics have been recognized as emerging pollutants with potential ecotoxicological impact. The contribution of washing machine use to microplastics emission at the household level is still not completely understood. This study aims to characterize microplastic emissions in laundry water from household washing machines from Greater Kuala Lumpur (Malaysia). Microplastics were found between 6.9E-3 and 0.183 g/m3 in laundry water at household level. Microplastic shapes of fiber and fragment consist of polyester, nylon, and acrylic with average length of 2258.59 μm and were also identified in these laundry water samples. Questionnaire survey findings demonstrated fabric properties and washing parameters both likely contribute to microplastic emissions in laundry water and, ultimately, wastewater treatment plant influent. The impact of fabric properties and washing parameter factors on microplastic emission in laundry water at the household level merits further investigation. The findings of this study demonstrated the potential of laundry water as a microplastic source at the household level within a developing country.
    Matched MeSH terms: Water; Water Purification; Waste Water
  4. Adsorption of Cu(II) and Ni(II) ions from wastewater onto bentonite and bentonite/GO composite
    Chang YS, Au PI, Mubarak NM, Khalid M, Jagadish P, Walvekar R, et al.
    Environ Sci Pollut Res Int, 2020 Sep;27(26):33270-33296.
    PMID: 32529626 DOI: 10.1007/s11356-020-09423-7
    Two superior adsorbents, namely bentonite and graphene oxide (GO), were hybridised to study the removal of copper and nickel ions from synthetic and industrial wastewater. The as-synthesised GO, bentonite/GO and bentonite were characterised by Fourier transform infrared spectroscopy, scanning electron microscopy, energy-dispersive X-ray spectroscopy and N2 adsorption-desorption analysis. The factors influencing the adsorption behaviours including contact time, initial solution pH, ionic strength, initial concentration of metal ions, temperature and adsorbent dosage were systematically investigated by batch equilibrium method. The adsorption equilibrium for copper and nickel onto bentonite was attained in 90 min while equilibrium was reached in 60 min on bentonite/GO. The adsorption of copper and nickel was pH-dependent in the range from pH 2 to pH 7 and from pH 2 to pH 8. Pseudo-first-order kinetic model excellently described the adsorption of copper and nickel onto bentonite and bentonite/GO. The equilibrium adsorption data was well described by the Langmuir isotherm model and the maximum adsorption capacity was 248.9 mg/g, 558.4 mg/g, 215.8 mg/g and 402.5 mg/g for bentonite-copper, bentonite/GO-copper, bentonite-nickel and bentonite/GO-nickel adsorption systems, respectively. The bentonite/GO composite exhibited a higher adsorption capacity of both cations from synthetic wastewater than pure bentonite owning to the synergistic effect between bentonite and GO. In all adsorption studies, copper was more efficiently removed than nickel due to its higher tendency to form bond with adsorbent surfaces. The adsorption of copper and nickel on bentonite/GO was mainly due to cation exchange, intermolecular and electrostatic interactions and physisorption dominated the adsorption processes. The practical application of bentonite/GO on adsorption of copper was investigated using real wastewater and its removal efficiency was beyond 98%. The excellent adsorption performances of composites for the copper and nickel removal from wastewater demonstrated its significant potential for pollution mitigations.
    Matched MeSH terms: Water Pollutants, Chemical/analysis*; Waste Water
  5. Adsorption of heavy metal from industrial wastewater onto low-cost Malaysian kaolin clay-based adsorbent
    Chai JB, Au PI, Mubarak NM, Khalid M, Ng WP, Jagadish P, et al.
    Environ Sci Pollut Res Int, 2020 Apr;27(12):13949-13962.
    PMID: 32036527 DOI: 10.1007/s11356-020-07755-y
    Adsorption capacity and percentage removal efficiency of Cu(II) and Ni(II) ions were studied and compared between raw kaolinite and acid-activated kaolinite. Acid-activated kaolin was prepared by refluxing raw kaolinite with concentrated sulphuric acid followed by calcination to enhance its surface properties and adsorption ability. Both raw and acid-activated kaolinite samples were characterized by Fourier transform infrared spectroscopy, energy dispersive X-ray, scanning electron micrograph and zeta potential analysis. Upon acid treatment, acid-activated kaolinite was discovered to have altered chemical composition and larger BET surface area as compared with raw kaolinite. The batch adsorption studies on aqueous solution were performed under different factors such as contact time, pH condition, adsorbent dosage, initial metal ion concentration and temperature. The optimum condition was selected for each factor including a contact time of 60 min, pH of 7.0, adsorbent dosage of 0.1 g, initial metal ion concentration of 100 mg/L and temperature of 25 °C. Then, the adsorption studies on wastewater samples were carried out at the selected optimum conditions. Acid-activated kaolinite always had better adsorption capacity and percentage removal efficiency than raw kaolinite due to the increasing amount of negative charges on the adsorbent surface and the number of metal ion binding sites upon acid treatment. The adsorption kinetic obtained was well described by the pseudo-second-order model, whereas the adsorption isotherms obtained were well described by either the Freundlich or the Langmuir adsorption model. The results showed that acid-activated kaolinite adsorbent is a better option as a favourable and feasible commercial low-cost adsorbent for wastewater treatment.
    Matched MeSH terms: Water Pollutants, Chemical*; Waste Water
  6. Phytosphere purification of urban domestic wastewater
    Qu Y, Yang Y, Sonne C, Chen X, Yue X, Gu H, et al.
    Environ Pollut, 2023 Nov 01;336:122417.
    PMID: 37598935 DOI: 10.1016/j.envpol.2023.122417
    Industrialization and overpopulation have polluted aquatic environments with significant impacts on human health and wildlife. The main pollutants in urban sewage are nitrogen, phosphorus, heavy metals and organic pollutants, which need to be treated with sewage, and the use of aquatic plants to purify wastewater has high efficiency and low cost. However, the effectiveness and efficiency of phytoremediation are also affected by temperature, pH, microorganisms and other factors. The use of biochar can reduce the cost of wastewater purification, and the combination of biochar and nanotechnology can improve the efficiency of wastewater purification. Some aquatic plants can enrich pollutants in wastewater, so it can be considered to plant these aquatic plants in constructed wetlands to achieve the effect of purifying wastewater. Biochar treatment technology can purify wastewater with high efficiency and low cost, and can be further applied to constructed wetlands. In this paper, the latest research progress of various pollutants in wastewater purification by aquatic plants is reviewed, and the efficient treatment technology of wastewater by biochar is discussed. It provides theoretical basis for phytoremediation of urban sewage pollution in the future.
    Matched MeSH terms: Water Purification*; Waste Water
  7. Integrating of electrocoagulation process with submerged membrane bioreactor for wastewater treatment under low voltage gradients
    Bani-Melhem K, Elektorowicz M, Tawalbeh M, Al Bsoul A, El Gendy A, Kamyab H, et al.
    Chemosphere, 2023 Oct;339:139693.
    PMID: 37536541 DOI: 10.1016/j.chemosphere.2023.139693
    Treating and reusing wastewater has become an essential aspect of water management worldwide. However, the increase in emerging pollutants such as polycyclic aromatic hydrocarbons (PAHs), which are presented in wastewater from various sources like industry, roads, and household waste, makes their removal difficult due to their low concentration, stability, and ability to combine with other organic substances. Therefore, treating a low load of wastewater is an attractive option. The study aimed to address membrane fouling in the submerged membrane bioreactor (SMBR) used for wastewater treatment. An aluminum electrocoagulation (EC) device was combined with SMBR as a pre-treatment to reduce fouling. The EC-SMBR process was compared with a conventional SMBR without EC, fed with real grey water. To prevent impeding biological growth, low voltage gradients were utilized in the EC deviceThe comparison was conducted over 60 days with constant transmembrane pressure and infinite solid retention time (SRT). In phase I, when the EC device was operated at a low voltage gradient (0.64 V/cm), no significant improvement in the pollutants removal was observed in terms of color, turbidity, and chemical oxygen demand (COD). Nevertheless, during phase II, a voltage gradient of 1.26 V/cm achieved up to 100%, 99.7%, 92%, 94.1%, and 96.5% removals in the EC-SMBR process in comparison with 95.1%, 95.4%, 85%, 91.7% and 74.2% removals in the SMBR process for turbidity, color, COD, ammonia nitrogen (NH3-N), total phosphorus (TP), respectively. SMBR showed better anionic surfactant (AS) removal than EC-SMBR. A voltage gradient of 0.64 V/cm in the EC unit significantly reduced fouling by 23.7%, while 1.26 V/cm showed inconsistent results. Accumulation of Al ions negatively affected membrane performance. Low voltage gradients in EC can control SMBR fouling if Al concentration is controlled. Future research should investigate EC-SMBR with constant membrane flux for large-scale applications, considering energy consumption and operating costs.
    Matched MeSH terms: Water/chemistry; Waste Water
  8. Fabrication of magnetic chitosan-grafted salicylaldehyde/nanoclay for removal of azo dye: BBD optimization, characterization, and mechanistic study
    Arni LA, Hapiz A, Jawad AH, Abdulhameed AS, ALOthman ZA, Wilson LD
    Int J Biol Macromol, 2023 Sep 01;248:125943.
    PMID: 37482164 DOI: 10.1016/j.ijbiomac.2023.125943
    Herein, a novel nanohybrid composite of magnetic chitosan-salicylaldehyde/nanoclay (MCH-SAL/NCLA) was hydrothermally synthesized for removal of azo dye (acid red 88, AR88) from simulated wastewater. Response surface methodology combined with the Box-Behnken design (RSM-BBD) was applied with 29 experiments to assess the impact of adsorption variables, that include A: % NCLA loading (0-50), B: MCH-SAL/NCLA dose (0.02-0.1 g/100 mL), C: pH (4-10), and time D: (10-90 min) on AR88 dye adsorption. The highest AR88 removal (75.16 %) as per desirability function was attained at the optimum conditions (NCLA loading = 41.8 %, dosage = 0.06 g/100 mL, solution pH = 4, and time = 86. 17 min). The kinetic and equilibrium adsorption results of AR88 by MCH-SAL/NCLA reveal that the process follows the pseudo-first-order and Temkin models. The MCH-SAL/NCLA composite has a maximum adsorption capacity (173.5 mg/g) with the AR88 dye. The adsorption of AR88 onto the MCH-SAL/NCLA surface is determined by a variety of processes, including electrostatic, hydrogen bonding, n-π, and n-π interactions. This research revealed that MCH-SAL/NCLA can be used as a versatile and efficient bio-adsorbent for azo dye removal from contaminated wastewater.
    Matched MeSH terms: Water Pollutants, Chemical*; Waste Water
  9. Ecological risk and source apportionment of heavy metals in surface water and sediments on Saint Martin's Island in the Bay of Bengal
    Sarker KK, Bristy MS, Alam N, Baki MA, Shojib FH, Quraishi SB, et al.
    Environ Sci Pollut Res Int, 2020 Sep;27(25):31827-31840.
    PMID: 32504432 DOI: 10.1007/s11356-020-09384-x
    The study aimed to determine eight hazardous heavy metals in surface water and sediment samples collected from the Naf River, Shah Porir Dwip (estuary), and mostly around Saint Martin's Island in the Bay of Bengal. The results of heavy metals in water samples were ranged as Pb 14.7-313.0, Cd 33.0-70.0, Cr
    Matched MeSH terms: Water; Water Pollutants, Chemical/analysis*
  10. Fulltext Prevalence and risk factors of childhood diarrhea among wastewater irrigating urban farming households in Addis Ababa
    Ali AS, Gari SR, Goodson ML, Walsh CL, Dessie BK, Ambelu A
    PLoS One, 2023;18(11):e0288425.
    PMID: 37939075 DOI: 10.1371/journal.pone.0288425
    INTRODUCTION: Childhood diarrhea is one of the major contributors to the morbidity of under-five children in Ethiopia. Although researchers determine the risk factors varyingly, the exposure route to the pathogens is usually complicated. This study aims to investigate the prevalence and risk factors of diarrhea among children under the age of five among wastewater irrigation farming households in Addis Ababa, Ethiopia.

    METHODS: Cross-sectional study was conducted among 402 farming households from November 2021 to February 2022. Data was collected using a face-to-face interviewer-administered questionnaire. Stata version 14 software was used to analyze data. Factors associated with the prevalence of diarrhea was identified using binary logistic regression. Multivariable analysis was carried out to determine an adjusted odds ratio at a confidence level of 95% and level of significance at 0.05.

    RESULTS: The overall prevalence of under-five children diarrheal cases was 22.3%. The odds of diarrhea are associated with a multitude of variables. Major wastewater-related determinants associated with diarrhea are body washing with irrigation water [AOR: 37.7, 95%CI (3.1, 358)], contaminated cloth with irrigation water [AOR:10.8,95%CI(0.6, 205)], use of protective clothing during farm work [28.9,95%CI (3.9, 215)], use of farm work cloths at home [AOR: 31.7, 95%CI (4.4, 226)], and bringing unwashed farm tools to home [94 (5.7, 1575)].

    CONCLUSION: The high prevalence of under-five children diarrheal disease among wastewater irrigation households was strongly associated with factors related to occupational exposure. Thus, to decrease childhood diarrheal among urban agriculture farmers, appropriate precautions need to be taken.

    Matched MeSH terms: Water; Waste Water*
  11. Growth enhancement of effective microorganisms for bioremediation of crude oil contaminated waters
    Mukred AM, Abd-Hamid A, Hamzah A, Yusoff WM
    Pak J Biol Sci, 2008 Jul 01;11(13):1708-12.
    PMID: 18819623
    The bioremediation of polluted groundwater, wastewater aeration pond and biopond sites was investigated using bacteria isolated from these sites located at the oil refinery Terengganu Malaysia. Out of 62 isolates, only 16 isolates from groundwater (8) and wastewater aeration pond (3) and biopond (5) were chosen based on growth medium containing 1% (v/v) Tapis crude oil. Only four isolates; Acinetobacter faecalis, Staphylococcus sp., Pseudomonas putida and Neisseria elongata showed percentage biodegradation of crude oil more than 50% after 5 days using Mineral Salts Medium (MSM). The effect of physical parameters (temperature, pH and agitation) on growth by all four strains showed a maximum growth in MSM medium with 1% Tapis crude oil at 37 degrees C with pH 7 and agitation of 130 rpm.
    Matched MeSH terms: Water Microbiology; Water Pollution, Chemical/analysis*
  12. Heavy metal (Cu2+) removal from wastewater by metal-organic framework composite adsorbent: Simulation-based- artificial neural network and response surface methodology
    Han F, Hessen AS, Amari A, Elboughdiri N, Zahmatkesh S
    Environ Res, 2024 Mar 15;245:117972.
    PMID: 38141913 DOI: 10.1016/j.envres.2023.117972
    Metal-organic framework (MOF)--based composites have received significant attention in a variety of applications, including pollutant adsorption processes. The current investigation was designed to model, forecast, and optimize heavy metal (Cu2+) removal from wastewater using a MOF nanocomposite. This work has been modeled by response surface methodology (RSM) and artificial neural network (ANN) algorithms. In addition, the optimization of the mentioned factors has been performed through the RSM method to find the optimal conditions. The findings show that RSM and ANN can accurately forecast the adsorption process's the Cu2+ removal efficiency (RE). The maximum values of RE are achieved at the highest value of time (150 min), the highest value of adsorbent dosage (0.008 g), and the highest value of pH (=6). The R2 values obtained were 0.9995, 0.9992, and 0.9996 for ANN modeling of adsorption capacity based on different adsorbent dosages, Cu2+ solution pHs, and different ion concentrations, respectively. The ANN demonstrated a high level of accuracy in predicting the local minima of the graph. In addition, the RSM optimization results showed that the optimum mode for RE occurred at an adsorbent dosage value of 0.007 g and a time value of 144.229 min.
    Matched MeSH terms: Water Pollutants, Chemical*; Waste Water
  13. Effects of Empagliflozin on Fluid Overload, Weight, and Blood Pressure in CKD
    Mayne KJ, Staplin N, Keane DF, Wanner C, Brenner S, Cejka V, et al.
    J Am Soc Nephrol, 2024 Feb 01;35(2):202-215.
    PMID: 38082486 DOI: 10.1681/ASN.0000000000000271
    SIGNIFICANCE STATEMENT: SGLT2 inhibitors reduce risk of kidney progression, AKI, and cardiovascular disease, but the mechanisms of benefit are incompletely understood. Bioimpedance spectroscopy can estimate body water and fat mass. One quarter of the EMPA-KIDNEY bioimpedance substudy CKD population had clinically significant levels of bioimpedance-derived "Fluid Overload" at recruitment. Empagliflozin induced a prompt and sustained reduction in "Fluid Overload," irrespective of sex, diabetes, and baseline N-terminal pro B-type natriuretic peptide or eGFR. No significant effect on bioimpedance-derived fat mass was observed. The effects of SGLT2 inhibitors on body water may be one of the contributing mechanisms by which they mediate effects on cardiovascular risk.

    BACKGROUND: CKD is associated with fluid excess that can be estimated by bioimpedance spectroscopy. We aimed to assess effects of sodium glucose co-transporter 2 inhibition on bioimpedance-derived "Fluid Overload" and adiposity in a CKD population.

    METHODS: EMPA-KIDNEY was a double-blind placebo-controlled trial of empagliflozin 10 mg once daily in patients with CKD at risk of progression. In a substudy, bioimpedance measurements were added to the main trial procedures at randomization and at 2- and 18-month follow-up visits. The substudy's primary outcome was the study-average difference in absolute "Fluid Overload" (an estimate of excess extracellular water) analyzed using a mixed model repeated measures approach.

    RESULTS: The 660 substudy participants were broadly representative of the 6609-participant trial population. Substudy mean baseline absolute "Fluid Overload" was 0.4±1.7 L. Compared with placebo, the overall mean absolute "Fluid Overload" difference among those allocated empagliflozin was -0.24 L (95% confidence interval [CI], -0.38 to -0.11), with similar sized differences at 2 and 18 months, and in prespecified subgroups. Total body water differences comprised between-group differences in extracellular water of -0.49 L (95% CI, -0.69 to -0.30, including the -0.24 L "Fluid Overload" difference) and a -0.30 L (95% CI, -0.57 to -0.03) difference in intracellular water. There was no significant effect of empagliflozin on bioimpedance-derived adipose tissue mass (-0.28 kg [95% CI, -1.41 to 0.85]). The between-group difference in weight was -0.7 kg (95% CI, -1.3 to -0.1).

    CONCLUSIONS: In a broad range of patients with CKD, empagliflozin resulted in a sustained reduction in a bioimpedance-derived estimate of fluid overload, with no statistically significant effect on fat mass.

    TRIAL REGISTRATION: Clinicaltrials.gov: NCT03594110 ; EuDRACT: 2017-002971-24 ( https://eudract.ema.europa.eu/ ).

    Matched MeSH terms: Water; Water-Electrolyte Imbalance*
  14. Fulltext Toxicity of metals to a freshwater snail, Melanoides tuberculata
    Shuhaimi-Othman M, Nur-Amalina R, Nadzifah Y
    ScientificWorldJournal, 2012;2012:125785.
    PMID: 22666089 DOI: 10.1100/2012/125785
    Adult freshwater snails Melanoides tuberculata (Gastropod, Thiaridae) were exposed for a four-day period in laboratory conditions to a range of copper (Cu), cadmium (Cd), zinc (Zn), lead (Pb), nickel (Ni), iron (Fe), aluminium (Al), and manganese (Mn) concentrations. Mortality was assessed and median lethal times (LT₅₀) and concentrations (LC₅₀) were calculated. LT₅₀ and LC₅₀ increased with the decrease in mean exposure concentrations and times, respectively, for all metals. The LC(50) values for the 96-hour exposures to Cu, Cd, Zn, Pb, Ni, Fe, Al, and Mn were 0.14, 1.49, 3.90, 6.82, 8.46, 8.49, 68.23, and 45.59 mg L⁻¹, respectively. Cu was the most toxic metal to M. tuberculata, followed by Cd, Zn, Pb, Ni, Fe, Mn, and Al (Cu > Cd > Zn > Pb > Ni > Fe > Mn > Al). Metals bioconcentration in M. tuberculata increases with exposure to increasing concentrations and Cu has the highest accumulation (concentration factor) in the soft tissues. A comparison of LC₅₀ values for metals for this species with those for other freshwater gastropods reveals that M. tuberculata is equally sensitive to metals.
    Matched MeSH terms: Fresh Water; Water Pollutants, Chemical/toxicity*
  15. Assessment of the microbial electrochemical sensor (SENTRY™) as a potential wastewater quality monitoring tool for common pollutants found in Malaysia
    Me MFH, Ang WL, Othman AR, Mohammad AW, Nasharuddin AAA, Aris AM, et al.
    Environ Monit Assess, 2024 Mar 14;196(4):366.
    PMID: 38483639 DOI: 10.1007/s10661-024-12526-0
    Bioelectrochemical sensors for environment monitoring have the potential to provide facility operators with real-time data, allowing for better and more timely decision-making regarding water and wastewater treatment. To assess the robustness and sensitivity of the Sentry™ biosensor in local conditions, it was tested in Malaysia using domestically available wastewater. The study objectives included (1) enrich the biosensor locally, (2) operate and test the biosensor with local domestic wastewater, and (3) determine the biosensor's responsiveness to model pollutants through pollutant spike and immersion test as well as response to absence of wastewater. Lab-scale operation shows the biosensor was successfully enriched with (1) local University Kebangsaan Malaysia's, microbial community strain collection and (2) local municipal wastewater microflora, operated for more than 50 days with a stable yet responsive carbon consumption rate (CCR) signal. Meanwhile, two independent biosensors were also enriched and operated in Indah Water Research Centre's crude sewage holding tank, showing a stable response to the wastewater. Next, a pilot scale setup was constructed to test the enriched biosensors for the spiked-pollutant test. The biosensors showed a proportional CCR response (pollutant presence detected) towards several organic compounds in the sewage, including ethanol, chicken blood, and dilution of tested sewage but less to curry powder, methanol, and isopropanol. Conversely, there was no significant response (pollutant presence not detected) towards hexane, Congo red, engine oil, and paint, which may be due to their non-biodegradability and/or insoluble nature. Additionally, the biosensors were exposed to air for 6 h to assess their robustness towards aerobic shock with a positive result. Overall, the study suggested that the biosensor could be a powerful monitoring tool, given its responsiveness towards organic compounds in sewage under normal conditions.
    Matched MeSH terms: Water; Waste Water*
  16. Effective adsorption of cadmium and lead using SO3H-functionalized Zr-MOFs in aqueous medium
    Gul S, Ahmad Z, Asma M, Ahmad M, Rehan K, Munir M, et al.
    Chemosphere, 2022 Nov;307(Pt 1):135633.
    PMID: 35810866 DOI: 10.1016/j.chemosphere.2022.135633
    Cadmium (Cd) and Lead (Pb) from industrial wastewater can bioaccumulate in the living organisms of water bodies, posing serious threats to human health. Therefore, efficient remediation of heavy metal ions of Cd (II) and Pb (II) in aqueous media is necessary for public health and environmental sustainability. In the present study, water stable Zirconium (Zr) based metal organic frameworks (MOFs) with SO3H functionalization were synthesized by solvothermal method and used first time for the adsorption of Cd (II) and Pb (II). Synthesis of UiO-66-SO3H, nano-sized (<100 nm) MOFs, was confirmed by FTIR, XRD, FESEM and BET. Effects of contact time, pH and temperature were investigated for adsorption of Cd (II) and Pb (II) onto SO3H-functionalized Zr-MOFs. The UiO-66-SO3H displayed notable rejections of 97% and 88% towards Cd (II) and Pb (II), respectively, after 160 min at 25 °C and pH (6) with an initial concentration of 1000 mg/L. Adsorption capacities of Cd (II) and Pb (II) were achieved as 194.9154 (mg/g) and 176.6879 (mg/g), respectively, at an initial concentration of 1000 mg/L. The Pseudo second-order kinetic model fitted well with linear regression (R2) of value 1. The mechanism was confirmed mainly as a chemisorption and coordination interaction between sulfone group (-SO3H) and metal ions Cd (IIa) and Pb (II). These results may support effective adsorption and can be studied further to enrich and recycle other heavy metals from wastewater.
    Matched MeSH terms: Water; Waste Water/chemistry
  17. Recent advancements in bamboo nanocellulose-based bioadsorbents and their potential in wastewater applications: A review
    Othman JAS, Ilyas RA, Nordin AH, Ngadi N, Alkbir MFM
    Int J Biol Macromol, 2024 Oct;277(Pt 3):134451.
    PMID: 39102907 DOI: 10.1016/j.ijbiomac.2024.134451
    The research interest in sustainable and eco-friendly materials based on natural sources has increased dramatically due to their recyclability, biodegradability, compatibility, and nontoxic behavior. Recently, nanocellulose-based green composites are under extensive exploration and have gained popularity among researchers owing to their lightweight, lost cost, low density, excellent mechanical and physical characteristics. This review provides a comprehensive overview of the recent advancements in the extraction, modification, and application of bamboo nanocellulose as a high-performance bioadsorbent. Bamboo, a rapidly renewable resource, offers an eco-friendly alternative to traditional materials due to its abundant availability and unique structural properties. Significantly, bamboo comprises a considerable amount of cellulose, approximately 40 % to 50%, rendering it a valuable source of cellulose fiber for the fabrication of cellulose nanocrystals. The review highlights different various modification techniques which enhance the adsorption capacities and selectivity of bamboo nanocellulose. Furthermore, the integration of bamboo nanocellulose into novel composite materials and its performance in removing contaminants such as heavy metals, dyes, and organic pollutants from wastewater are critically analyzed. Emphasis is placed on the mechanisms of adsorption, regeneration potential, and the economic and environmental benefits of using bamboo-based bioadsorbents. The findings underscore the potential of bamboo nanocellulose to play a pivotal role in developing sustainable wastewater treatment technologies, offering a promising pathway towards cleaner water and a greener future.
    Matched MeSH terms: Water Pollutants, Chemical/isolation & purification; Water Pollutants, Chemical/chemistry
  18. Fulltext Potential biosorbent derived from Calligonum polygonoides for removal of methylene blue dye from aqueous solution
    Nasrullah A, Khan H, Khan AS, Man Z, Muhammad N, Khan MI, et al.
    ScientificWorldJournal, 2015;2015:562693.
    PMID: 25705714 DOI: 10.1155/2015/562693
    The ash of C. polygonoides (locally called balanza) was collected from Lakki Marwat, Khyber Pakhtunkhwa, Pakistan, and was utilized as biosorbent for methylene blue (MB) removal from aqueous solution. The ash was used as biosorbent without any physical or chemical treatment. The biosorbent was characterized by using various techniques such as Fourier transform infrared spectroscopy (FTIR), thermogravimetric analysis (TGA), and scanning electron microscopy (SEM). The particle size and surface area were measured using particle size analyzer and Brunauer-Emmett-Teller equation (BET), respectively. The SEM and BET results expressed that the adsorbent has porous nature. Effects of various conditions such as initial concentration of methylene blue (MB), initial pH, contact time, dosage of biosorbent, and stirring rate were also investigated for the adsorption process. The rate of the adsorption of MB on biomass sample was fast, and equilibrium has been achieved within 1 hour. The kinetics of MB adsorption on biosorbent was studied by pseudo-first- and pseudo-second-order kinetic models and the pseudo-second-order has better mathematical fit with correlation coefficient value (R (2)) of 0.999. The study revealed that C. polygonoides ash proved to be an effective, alternative, inexpensive, and environmentally benign biosorbent for MB removal from aqueous solution.
    Matched MeSH terms: Water Pollutants, Chemical/isolation & purification*; Water Pollutants, Chemical/metabolism; Water Pollutants, Chemical/chemistry; Water Purification/methods*
  19. Water quality assessment of an unusual ritual well in Bangladesh and impact of mass bathing on this quality
    Zabed H, Suely A, Faruq G, Sahu JN
    Sci Total Environ, 2014 Feb 15;472:363-9.
    PMID: 24295752 DOI: 10.1016/j.scitotenv.2013.11.051
    A sacred ritual well with continuously discharging of methane gas through its water body was studied for physicochemical and microbiological quality in three seasons and during ritual mass bathing. Most of the physicochemical parameters showed significant seasonal variations (P<0.05) and a sharp fluctuation during mass bathing. Dissolved oxygen (DO) was found negatively correlated with temperature (r=-0.384, P<0.05), biochemical oxygen demand (BOD) (r=-0.58, P<0.001) and ammonia (r=-0.738, P<0.001), while BOD showed positive correlation with chemical oxygen demand (COD) (r=0.762, P<0.001) and ammonia (r=0.83, P<0.001). Simple regression analysis also yielded significant linear relationship in DO vs. temperature (r(2)=0.147, P<0.05), DO vs. ammonia (r(2)=0.544, P<0.001) and BOD vs. DO (r(2)=0.336, P<0.001). A total of eight microbial indicators were studied and found that all of them increased unusually during mass bathing comparing with their respective seasonal values. Total coliforms (TC) were found positively correlated with fecal coliforms (FC) (r=0.971), FC with Escherichia coli (EC) (r=0.952), EC with intestinal enterococci (IE) (r=0.921), fecal streptococci (FS) with IE (r=0.953) and Staphylococcus aureus (SA) with Pseudomonas aeruginosa (PA) (r=0.946), which were significant at P<0.001. Some regression models showed significant linear relationship at P<0.001 with r(2) value of 0.943 for FC vs. TC, 0.907 for EC vs. FC, 0.869 for FS vs. FC, 0.848 for IE vs. EC and 0.909 for IE vs. FS. The overall results found in this study revealed that well water is suitable for bathing purpose but the religious activity considerably worsen its quality.
    Matched MeSH terms: Water Microbiology*; Water Pollution/analysis*; Water Pollution/statistics & numerical data; Water Quality
  20. Determination of polar aromatic amines using newly synthesized sol-gel titanium (IV) butoxide cyanopropyltriethoxysilane as solid phase extraction sorbent
    Miskam M, Abu Bakar NK, Mohamad S
    Talanta, 2014 Mar;120:450-5.
    PMID: 24468395 DOI: 10.1016/j.talanta.2013.12.037
    A solid phase extraction (SPE) method has been developed using a newly synthesized titanium (IV) butoxide-cyanopropyltriethoxysilane (Ti-CNPrTEOS) sorbent for polar selective extraction of aromatic amines in river water sample. The effect of different parameters on the extraction recovery was studied using the SPE method. The applicability of the sorbents for the extraction of polar aromatic amines by the SPE was extensively studied and evaluated as a function of pH, conditioning solvent, sample loading volume, elution solvent and elution solvent volume. The optimum experimental conditions were sample at pH 7, dichloromethane as conditioning solvent, 10 mL sample loading volume and 5 mL of acetonitrile as the eluting solvent. Under the optimum conditions, the limit of detection (LOD) and limit of quantification (LOQ) for solid phase extraction using Ti-CNPrTEOS SPE sorbent (0.01-0.2; 0.03-0.61 µg L(-1)) were lower compared with those achieved using Si-CN SPE sorbent (0.25-1.50; 1.96-3.59 µg L(-1)) and C18 SPE sorbent (0.37-0.98; 1.87-2.87 µg L(-1)) with higher selectivity towards the extraction of polar aromatic amines. The optimized procedure was successfully applied for the solid phase extraction method of selected aromatic amines in river water, waste water and tap water samples prior to the gas chromatography-flame ionization detector separation.
    Matched MeSH terms: Water Pollutants, Chemical/analysis*; Drinking Water/analysis; Waste Water/analysis
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